more pop.
More pop, hunh? Well, I would do it by lightening up the bike. You can run without a battery or battery box, fit alloy rims and stainless spokes, and make thinks like spacers and whatnot out of alloy. Then lower your final drive gearing. I don't think that hot rodding the engine should be necessary for more "pop", although a camshaft with slightly more lift and a little different timing might compliment the 750 engine. Lighten the valve train, so that the internals aren't as stressed when you get over 6000 rpm.
Work with the strong suit of the long stroke engine....mid range torque. I would rather fit a five speed gearbox and a 19T final drive sprocket for street blasting than to build a conventional high compression cammy hot rod engine. Keep the revs down, but an extra cog in the gearbox will keep you in the sweet spot.
Alloy rims give you many advantages...less mass on the ends for better mass centralization, less mass to spin up to speed, less mass to accelerate linearly, less mass to slow during braking, less mass for the suspension to control, less mass to have to move out of the rotational plane when cornering...so easier steering. Plus they look great and don't rust. Start there, I suggest. Also, you then have the option of using 18" rubber on the rear, if you relace with a WM3X18 rim. Check
http://www.buchananspokes.com/
If you fit the 18" and use a 110/90/18 tire, the overall diameter will be slightly smaller than the 4.10 /19 stocker, slightly lowering the gearing, so try that before changing sprockets.