Well, I have a '71 750 and a '73 850, so may be able to weigh in. I prefer the '71's fork angle steering to the 850's. It steers quicker in the twisties, the 850 slightly less so. I didn't think it made much difference on the highway, even when taken to the top end, but that's lower on a 750 due to the 19 tooth gearbox output sprocket.
You will want to fix the sidestand mount. Rear shock reinforcement too. Both were available from Old Britts, but you better hurry, they're selling everything off for their retirement.
A '72 frame would be my choice if you wanted to use a 750 frame.